Global and regional trends of atmospheric sulfur

15728 9 86437 2 245201 document 86437 s41598-018-37304-0.pdf application/pdf 59cbd397f18ff1077a670ad114d18dbb MD5 3726331 2019-02-04 07:26:05 https://pure.iiasa.ac.at/id/eprint/15728/1/s41598-018-37304-0.pdf 15728 1 1 application/pdf text en public cc_by_4

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published 86438 1 245208 document 86438 indexcodes.txt text/x-asm d2fa7334e4e93232932c7ece17e802cc MD5 12031 2019-02-04 07:36:03 https://pure.iiasa.ac.at/id/eprint/15728/2/indexcodes.txt 15728 2 2 text/x-asm other Generate index codes conversion from text to indexcodes en public

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http://eprints.org/relation/isVersionOf https://pure.iiasa.ac.at/id/document/86437 http://eprints.org/relation/isVolatileVersionOf https://pure.iiasa.ac.at/id/document/86437 http://eprints.org/relation/ismediumThumbnailVersionOf https://pure.iiasa.ac.at/id/document/86437 86442 2 245212 document 86442 small.jpg image/png f9f5ea9847f06022693eff0cd55ae036 MD5 1971 2019-02-04 07:36:22 https://pure.iiasa.ac.at/id/eprint/15728/6/small.jpg 15728 6 6 image/png other Thumbnails conversion from text to thumbnail_small en public

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published 90489 2 261961 document 90489 lightbox.jpg image/png ea3175c2be69c1b081fe048bc99c26f0 MD5 50810 2020-06-05 11:35:46 https://pure.iiasa.ac.at/id/eprint/15728/8/lightbox.jpg 15728 8 8 image/png other Thumbnails conversion from text to thumbnail_lightbox en public

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http://eprints.org/relation/isVersionOf https://pure.iiasa.ac.at/id/document/90487 http://eprints.org/relation/isVolatileVersionOf https://pure.iiasa.ac.at/id/document/90487 http://eprints.org/relation/isIndexCodesVersionOf https://pure.iiasa.ac.at/id/document/90487 archive 353 disk0/00/01/57/28 2019-02-04 07:30:07 2021-08-27 17:31:23 2019-02-04 07:30:07 article show Aas W. Mortier A. Bowersox V. Cherian R. Faluvegi G. Fagerli H. Hand J. Klimont Z. 1473 0000-0003-2630-198X Galy-Lacaux C. Lehmann C.M.B. Myhre C.L. Myhre G. Olivié D. Sato K. Quaas J. Rao P.S.P. Schulz M. Shindell D. Skeie R.B. Stein A. Takemura T. Tsyro S. Vet R. Xu X. Global and regional trends of atmospheric sulfur pub prog_air The profound changes in global SO2 emissions over the last decades have affected atmospheric composition on a regional and global scale with large impact on air quality, atmospheric deposition and the radiative forcing of sulfate aerosols. Reproduction of historical atmospheric pollution levels based on global aerosol models and emission changes is crucial to prove that such models are able to predict future scenarios. Here, we analyze consistency of trends in observations of sulfur components in air and precipitation from major regional networks and estimates from six different global aerosol models from 1990 until 2015. There are large interregional differences in the sulfur trends consistently captured by the models and observations, especially for North America and Europe. Europe had the largest reductions in sulfur emissions in the first part of the period while the highest reduction came later in North America and East Asia. The uncertainties in both the emissions and the representativity of the observations are larger in Asia. However, emissions from East Asia clearly increased from 2000 to 2005 followed by a decrease, while in India a steady increase over the whole period has been observed and modelled. The agreement between a bottom-up approach, which uses emissions and process-based chemical transport models, with independent observations gives an improved confidence in the understanding of the atmospheric sulfur budget. 2019-01-30 published NPG 10.1038/s41598-018-37304-0 159 public Scientific Reports 9 1 e953 TRUE 2045-2322 Evaluating the Climate and Air Quality Impacts of Short-Lived Pollutants (ECLIPSE, FP7 282688) FALSE yes info:eu-repo/grantAgreement/EC/FP7/282688/EU/Evaluating the Climate and Air Quality Impacts of Short-Lived Pollutants/ECLIPSE info:eu-repo/semantics/article info:eu-repo/semantics/openAccess