Variability and quasi-decadal changes in the methane budget over the period 2000-2012

Saunois M, Bousquet P, Poulter B, Peregon A, Ciais P, Canadell JG, Dlugokencky EJ, Etiope G, et al. (2017). Variability and quasi-decadal changes in the methane budget over the period 2000-2012. Atmospheric Chemistry and Physics Discussions: 1-39. DOI:10.5194/acp-2017-296. (In Press)

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Project: Operational Global Carbon Observing System (GEOCARBON, FP7 283080), Predicting future methane fluxes from Northern lakes (METLAKE, H2020 725546), Monitoring Atmospheric Composition and Climate Interim Implementation (MACCII, FP7 283576), Monitoring Atmospheric Composition and Climate -III (MACCIII, H2020 633080), Carbon dioxide regulation of Earth’s ecological weathering engine: from microorganisms to ecosystems (CDREG, FP7 322998)

Abstract

Following the recent Global Carbon project (GCP) synthesis of the decadal methane (CH4) budget over 2000–2012 (Saunois et al., 2016), we analyse here the same dataset with a focus on quasi-decadal and inter-annual variability in CH4 emissions. The GCP dataset integrates results from top-down studies (exploiting atmospheric observations within an atmospheric inverse-modelling frameworks) and bottom-up models, inventories, and data-driven approaches (including process-based models for estimating land surface emissions and atmospheric chemistry, inventories of anthropogenic emissions, and data-driven extrapolations).

The annual global methane emissions from top-down studies, which by construction match the observed methane growth rate within their uncertainties, all show an increase in total methane emissions over the period 2000–2012, but this increase is not linear over the 13 years. Despite differences between individual studies, the mean emission anomaly of the top-down ensemble shows no significant trend in total methane emissions over the period 2000–2006, during the plateau of atmospheric methane mole fractions, and also over the period 2008–2012, during the renewed atmospheric methane increase. However, the top-down ensemble mean produces an emission shift between 2006 and 2008, leading to 22 [16–32] Tg CH4 yr−1 higher methane emissions over the period 2008–2012 compared to 2002–2006. This emission increase mostly originated from the tropics with a smaller contribution from mid-latitudes and no significant change from boreal regions.

The regional contributions remain uncertain in top-down studies. Tropical South America and South and East Asia seems to contribute the most to the emission increase in the tropics. However, these two regions have only limited atmospheric measurements and remain therefore poorly constrained.

The sectorial partitioning of this emission increase between the periods 2002–2006 and 2008–2012 differs from one atmospheric inversion study to another. However, all top-down studies suggest smaller changes in fossil fuel emissions (from oil, gas, and coal industries) compared to the mean of the bottom-up inventories included in this study. This difference is partly driven by a smaller emission change in China from the top-down studies compared to the estimate in the EDGARv4.2 inventory, which should be revised to smaller values in a near future. Though the sectorial partitioning of six individual top-down studies out of eight are not consistent with the observed change in atmospheric 13CH4, the partitioning derived from the ensemble mean is consistent with this isotopic constraint. At the global scale, the top-down ensemble mean suggests that, the dominant contribution to the resumed atmospheric CH4 growth after 2006 comes from microbial sources (more from agriculture and waste sectors than from natural wetlands), with an uncertain but smaller contribution from fossil CH4 emissions. Besides, a decrease in biomass burning emissions (in agreement with the biomass burning emission databases) makes the balance of sources consistent with atmospheric 13CH4 observations.

The methane loss (in particular through OH oxidation) has not been investigated in detail in this study, although it may play a significant role in the recent atmospheric methane changes.

Item Type: Article
Research Programs: Air Quality & Greenhouse Gases (AIR)
Mitigation of Air Pollution (MAG)
Depositing User: Luke Kirwan
Date Deposited: 16 May 2017 13:31
Last Modified: 16 May 2017 14:36
URI: http://pure.iiasa.ac.at/14598

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